38071
Author
Manning, M.R.; Lowe, D.C.; Melhuish, W.H.; Sparks, R.J.; Wallace, Gavin; Brenninkmeijer, C.A.M.; McGill, R.C.
Title Of Article Chaper
The use of radiocarbon measurements in atmospheric studies
Title Of Journal Book
Radiocarbon
Volume
32
Issue
1
Pages
37-58
Collation
3 tables, 6 figs.
Reference Bibliography
refs.
ISSN
0033-8222
Language Of Text
English
Language Of Summary
English
Literature Type
Serial
Literature Level
Analytic
Abstract
Carbon-14 measured in trace gases in clean air helps to determine the sources of such gases, their long-range transport in the atmosphere, and their exchange with other carbon cycle reservoirs. In order to separate sources, transport, and exchange, it is necessary to interpret measurements using models of these processes. Presents atmospheric <sup>14</sup>CO<sub>2</sub> measurements made in New Zealand since 1954 and at various Pacific Ocean sites for shorter periods. Analyzes these for latitudinal and seasonal variation, the latter being consistent with a seasonally varying exchange rate between the stratosphere and troposphere. The observed seasonal cycle does not agree with that predicted by a zonally averaged global circulation model. Discusses recent accelerator mass spectrometry measurements of atmospheric <sup>14</sup>CH<sub>4</sub> and the problems involved in determining the fossil fuel methane source. Current data imply a fossil carbon contribution of ca. 25%, and the major sources of uncertainty in this number are the uncertainty in the nuclear power source of <sup>14</sup>CH<sub>4</sub>, and in the measured value for delta<sup>14</sup>C in atmospheric methane.
Keywords
radiocarbon dating;carbon-14;atmosphere;New Zealand;seasonal; accelerator mass spectrometry;Pacific Ocean;methane
pub_id
38071